You can deploy and run Angular ASP.NET Core video chat applications on Microsoft Azure using Twilio Programmable Video, leveraging a fully managed enterprise-grade cloud platform for easy deployment and configuration. To get started, you'll need a GitHub account, Microsoft account, Azure account, Twilio account, Visual Studio 2017 or 2019, and access to the video chat project source code, which can be obtained from the author's GitHub repository or by following previous instructions to build it locally. Once you have your credentials set up, you can publish your application to Azure using Visual Studio, add your Twilio configuration credentials to app settings in Azure, and test your video chat application functionality in a browser.